http://purl.uniprot.org/citations/28718766 | http://www.w3.org/1999/02/22-rdf-syntax-ns#type | http://purl.uniprot.org/core/Journal_Citation |
http://purl.uniprot.org/citations/28718766 | http://www.w3.org/2000/01/rdf-schema#comment | "In plants, algae and cyanobacteria, Photosystem II (PSII) catalyzes the light-driven splitting of water at a protein-bound Mn4CaO5-cluster, the water-oxidizing complex (WOC). In the photosynthetic organisms, the light-driven formation of the WOC from dissolved metal ions is a key process because it is essential in both initial activation and continuous repair of PSII. Structural information is required for understanding of this chaperone-free metal-cluster assembly. For the first time, we obtained a structure of PSII from Thermosynechococcus elongatus without the Mn4CaO5-cluster. Surprisingly, cluster-removal leaves the positions of all coordinating amino acid residues and most nearby water molecules largely unaffected, resulting in a pre-organized ligand shell for kinetically competent and error-free photo-assembly of the Mn4CaO5-cluster. First experiments initiating (i) partial disassembly and (ii) partial re-assembly after complete depletion of the Mn4CaO5-cluster agree with a specific bi-manganese cluster, likely a di-µ-oxo bridged pair of Mn(III) ions, as an assembly intermediate."xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.org/dc/terms/identifier | "doi:10.7554/elife.26933"xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/author | "Zhang M."xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/author | "Bommer M."xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/author | "Dobbek H."xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/author | "Kern J."xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/author | "Zouni A."xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/author | "Dau H."xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/author | "Yano J."xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/author | "Chatterjee R."xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/author | "Hussein R."xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/date | "2017"xsd:gYear |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/name | "Elife"xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/pages | "e26933"xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/title | "Structural insights into the light-driven auto-assembly process of the water-oxidizing Mn4CaO5-cluster in photosystem II."xsd:string |
http://purl.uniprot.org/citations/28718766 | http://purl.uniprot.org/core/volume | "6"xsd:string |
http://purl.uniprot.org/citations/28718766 | http://www.w3.org/2004/02/skos/core#exactMatch | http://purl.uniprot.org/pubmed/28718766 |
http://purl.uniprot.org/citations/28718766 | http://xmlns.com/foaf/0.1/primaryTopicOf | https://pubmed.ncbi.nlm.nih.gov/28718766 |
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http://purl.uniprot.org/uniprot/#_P0A386-mappedCitation-28718766 | http://www.w3.org/1999/02/22-rdf-syntax-ns#object | http://purl.uniprot.org/citations/28718766 |
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http://purl.uniprot.org/uniprot/#_Q9F1L5-mappedCitation-28718766 | http://www.w3.org/1999/02/22-rdf-syntax-ns#object | http://purl.uniprot.org/citations/28718766 |